The idea behind Greyhole is to have all your shares on 1 drive, and use the others in the pool for redundency.
Not.
Greyhole can pool as many drives as you'd like, and give you one big share, with or without redundancy.
If you don't want redundancy, you just specify Extra copies = 0 (- I think in the drop-down menu in Amahi).
Typically the shares on the OS drive in /var/hda/files directory. The drives located in /var/hda/files/drives are the pool ones.
By default, /var/hda/files is what is called the landing zone, i.e. where the files end up when you copy them into share handled by Greyhole.
At that point, the Greyhole daemon will pick that file copy, and MOVE it into one of the drives you included in your pool, and leave behind only a symlink that takes next to no space.
How would I for example make my games folder here more than 1.8tb by pooling one or more of my other drives?
Add all your /var/hda/drives/driveXYZ to the storage pool, and check the "Uses Greyhole" for the share you want to use the pool.
If you connect to those shares from a remote computer, and check how much free space the share has, you'll see it has the sum of all the free space of the pooled drives.